Cary is a town in Wake, Chatham, and Durham counties in the U.S. state of North Carolina and is part of the Raleigh-Cary, NC Metropolitan Statistical Area. According to the 2020 census, its population was 174,721, making it the seventh-most populous municipality in North Carolina, and the 148th-most populous in the United States. In 2023, the town's po…Cary is a town in Wake, Chatham, and Durham counties in the U.S. state of North Carolina and is part of the Raleigh-Cary, NC Metropolitan Statistical Area. According to the 2020 census, its population was 174,721, making it the seventh-most populous municipality in North Carolina, and the 148th-most populous in the United States. In 2023, the town's population had increased to 180,010.